He is also known for starring in the films The Covenant (2006), The Haunting of Molly Hartley (2008), Twelve (2010), and What to Expect When You're Expecting (2012).
In 2008, Crawford co-starred in the crime-thriller Loaded, and portrayed the lead role in the supernatural horror film The Haunting of Molly Hartley.
The following year, he played English singer-songwriter Leona Lewis' boyfriend in the video for her single "I Will Be", which was released in January 2009.
However, Taylor Momsen and Chace Crawford denied the fact that they were dating, Momsen personally thinks of Chace as a really good friend, but nothing more.
Taylor Momsen and Leighton Meester are also really good friends in the real life, which is unexpected as they were world’s biggest enemies on TV series.
She is strong, passionate about her music; she is provocative and sometimes even rude.